分类： 光学 >> 量子光学 提交时间： 2023-02-19
摘要： Missing second-order nonlinearity in centrosymmetric graphene overshadows its intriguing optical attribute. Here, we report redox-governed charge doping could effectively break the centrosymmetry of bilayer graphene (BLG), enabling a strong second harmonic generation (SHG) with a strength close to that of the well-known monolayer MoS2. Verified from control experiments with in situ electrical current annealing and electrically gate-controlled SHG, the required centrosymmetry breaking of the emerging SHG arises from the charge-doping on the bottom layer of BLG by the oxygen/water redox couple. Our results not only reveal that charge doping is an effective way to break the inversion symmetry of BLG despite its strong interlayer coupling but also indicate that SHG spectroscopy is a valid technique to probe molecular doping on two-dimensional materials.
分类： 光学 >> 量子光学 提交时间： 2023-02-19
摘要： High resolution images are widely used in our daily life, whereas high-speed video capture is challenging due to the low frame rate of cameras working at the high resolution mode. Digging deeper, the main bottleneck lies in the low throughput of existing imaging systems. Towards this end, snapshot compressive imaging (SCI) was proposed as a promising solution to improve the throughput of imaging systems by compressive sampling and computational reconstruction. During acquisition, multiple high-speed images are encoded and collapsed to a single measurement. After this, algorithms are employed to retrieve the video frames from the coded snapshot. Recently developed Plug-and-Play (PnP) algorithms make it possible for SCI reconstruction in large-scale problems. However, the lack of high-resolution encoding systems still precludes SCI's wide application. In this paper, we build a novel hybrid coded aperture snapshot compressive imaging (HCA-SCI) system by incorporating a dynamic liquid crystal on silicon and a high-resolution lithography mask. We further implement a PnP reconstruction algorithm with cascaded denoisers for high quality reconstruction. Based on the proposed HCA-SCI system and algorithm, we achieve a 10-mega pixel SCI system to capture high-speed scenes, leading to a high throughput of 4.6G voxels per second. Both simulation and real data experiments verify the feasibility and performance of our proposed HCA-SCI scheme.
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